The support of a measure is the intersection of all closed sets that have full measure. This means that if a measure $\mu$ is concentrated on a set $A$, the inclusion $\operatorname{supp}(\mu) \subset \overline{A}$ holds [if $\mu$ is at least $\sigma$-finite].
This is pretty much all you can say about the set-theoretic relation between those two sets. Take for example the Lebesgue-measure. It's support is $\mathbb{R}$, but it is concentrated on every set of the form $\mathbb{R} \setminus \\{x\\}$. You can remove any element from $\mathbb{R}$ and the Lebesgue-measure is still concentrated on this "narrowed" set. But the support is uniquely determined as $\mathbb{R}$.