Because you used the permanent parameter you can only revert manually by deleting the same entry.
ip -6 neighbour delete fe80::1 lladdr 28:99:3a:4d:23:91 dev eth0 nud permanent
I am not aware of why your VPS provider is telling you to do this if IPv6 was accessible before.
To get back to an autoconfigured state without restarting type
ip -6 neighbour flush
ip -6 neighbour
That gets you stateless IPv6. If its still not getting an IP try
dhclient -6
If that doesn't work you need more information from your VPS provider.